欢迎访问中国科学院大学学报,今天是
大气颗粒物与空气污染专刊

杭州市区污染物消光特性研究

  • 洪盛茂 ,
  • 徐昶 ,
  • 沈建东 ,
  • 焦荔 ,
  • 何曦 ,
  • 杨乐 ,
  • 孙鸿良 ,
  • 徐鸿 ,
  • 叶贤满 ,
  • 张天 ,
  • 何纪平 ,
  • 姚晗
展开
  • 杭州市环境监测中心站, 杭州 310007

收稿日期: 2013-03-11

  修回日期: 2013-11-15

  网络出版日期: 2014-05-15

基金资助

杭州市重大科技创新项目(20092113A05)、浙江省重大科技专项重点社会发展项目(2011C13022)资助

Research of pollutants extinction characteristic in Hangzhou

  • HONG Shengmao ,
  • XU Chang ,
  • SHEN Jiandong ,
  • JIAO Li ,
  • HE Xi ,
  • YANG Le ,
  • SUN Hongliang ,
  • XU Hong ,
  • YE Xianman ,
  • ZHANG Tian ,
  • HE Jiping ,
  • YAO Han
Expand
  • Hangzhou Environmental Monitoring Center Station, Hangzhou 310007, China

Received date: 2013-03-11

  Revised date: 2013-11-15

  Online published: 2014-05-15

摘要

利用美国IMPROVE能见度公式,分析2011年6月至2012年5月杭州大气复合污染综合监测数据,研究污染物的消光特征,确定首要消光物质.研究结果表明,随着能见度降低,污染物消光系数在大气总消光系数中的比例逐渐减少,从10km处的85%左右降低到2km以下的22%左右.与10km处相比,2km处的NO3-和SO42-消光系数分别增长3.43倍和2.15倍.杭州污染物质的消光系数具有非常明显的季节变化和日变化特征,硝酸盐表现为夏季较低,冬季较高;硫酸盐表现为秋季高,其他3季相对较低.

本文引用格式

洪盛茂 , 徐昶 , 沈建东 , 焦荔 , 何曦 , 杨乐 , 孙鸿良 , 徐鸿 , 叶贤满 , 张天 , 何纪平 , 姚晗 . 杭州市区污染物消光特性研究[J]. 中国科学院大学学报, 2014 , 31(3) : 360 -366 . DOI: 10.7523/j.issn.2095-6134.2014.03.010

Abstract

Using the visibility formula of IMPROVE, the data of atmospheric complex pollution monitoring system in Hangzhou from July 2011 to June 2012 was analysed. The primary extinction material was determined. The results showed that the ratio of pollutant extinction coefficient to atmospheric total extinction coefficient decreased when the visibility decreased, and the ratio decreased from 85% at 10 km to 22% at below 2 km. The extinction coefficients of nitrate and sulfate at below 2 km were 4.43 and 3.15 times of those at 10 km, respectively. The extinction coefficients of main pollutants in Hangzhou showed very significant seasonal variation and daily variation. The extinction coefficient of nitrate was lower in summer and autumn and higher in winter and spring, while the extinction coefficient of sulfate was higher in autumn and lower in the other seasons.

参考文献

[1] 国家环境保护局, 国家技术监督局. 环境空气质量标准(GB3095—1996)[S]. 北京:中国环境科学出版社,1996.

[2] 环境保护部, 国家质量监督检验检疫总局. 环境空气质量标准(GB3095—2012)[S].北京:中国环境科学出版社,2012.

[3] 国家气象局.霾的观测与预报等级(QX/T—2010)[S].北京:气象出版社,2010.

[4] Hong S M. The influence of air ozone concentration in air pollution index(API) Hangzhou urban[J]. Environmental Monitoring in China. 2010, 26(1):46-52(in Chinese). 洪盛茂. 杭州主城区大气臭氧对空气污染指数API的影响[J]. 中国环境监测, 2010, 26(1):46-52.

[5] Xue Z G,Liu Y,Chai F H, et al. Schemes and demonstrations for air pollution index improvement[J]. Research of Environmental Sciences,2011,24(2):125-132(in Chinese). 薛志钢, 刘妍, 柴发合,等. 城市空气污染指数改进方案及论证[J]. 环境科学研究,2011,24(2):125-132.

[6] Zhang Y N, Li Q Q, Luo Y K, et al. Regional air quality index in the Pearl River Delta[J]. Environmental Science & Technology. 2010, 33(3):9-13(in Chinese). 张轶男, 李倩倩, 罗运阔,等. 珠三角区域空气质量指数(RAQI)的研究[J]. 环境科学与技术, 2010, 33(3):9-13.

[7] Duan J C,Xue Z G,Chai F H, et al. Correlation between public sentiment and air pollution index in two typical cities in China[J]. Research of Environmental Sciences, 2011,24(2):133-138(in Chinese). 段菁春, 薛志钢, 柴发合,等. 典型城市公众感受与空气污染指数的相关关系[J]. 环境科学研究, 2011,24(2):133-138.

[8] Tao J,Zhang R J,Xu Z C, et al. Contribution factors of ambient light extinction coefficient in the winter of Guangzhou[J]. Climatic and Environmental Research,2009, 14 (5): 484-490.(in Chinese) 陶俊, 张仁健, 许振成, 等. 广州冬季大气消光系数的贡献因子研究[J]. 气候与环境研究, 2009,14 ( 5): 484-490.

[9] Li L J, Wang Y, Li J X, et al. The characteristic of atmospheric particle size distribution and their light extinction effect in Beijing during winter and spring time[J]. Research of Environmental Sciences, 2008,21(2):90-94.(in Chinese) 李令军,王英,李金香,等.北京市冬春季大气颗粒物的粒径分布及消光作用[J].环境科学研究,2008,21(2):90-94.

[10] Li X B, Xu Q S, Wei H L, et al. Study on relationship between extinction coefficient and mass concentration[J]. Acta Optica Sinica, 2008, 28(9):1655-1658(in Chinese). 李学彬,徐青山,魏合理,等.气溶胶消光系数与质量浓度的相关性研究[J].光学学报,2008,28(9):1655-1658.

[11] Liu X M, Shao M. The analysis of sources of ambient light extinction coefficient in summer time of Beijing city[J]. Acta Scientiae Circumstantiae,2004,24(2):185-189(in Chinese). 刘新民, 邵敏.北京市夏季大气消光系数的来源分析[J].环境科学学报, 2004, 24(2):185-189.

[12] Hand J L, Copeland S A, Day D K, et al.Spatial and seasonal patterns and temporal variability of haze and its constituents in the united states report V.ISSN 0737-5352-87. Improve Report V. 5.1-23,2011.

[13] Appel B R, Tokiwa Y, Hsu J, et al. Visibility as relation to atmospheric aerosol constituents[J]. Atmospheric Enviroment, 1985, 19(9):1525-1534.

[14] Li L, Chen J M, Wang L,et al. Aerosol single scattering albedo affected by chemical composition: an investigation using CRDS combined with MARGA[J]. Atmospheric Research,2013, 124:149-157.

[15] Thompson J E, Hayes P L, Jimenez J L, et al. Aerosol optical properties at Pasadena, CA during CalNex 2010[J]. Atmospheric Enviroment,2012, 55:190-200.

[16] Malm W C, Molenar J V, Eldred R A, et al. Examining the relationship among atmospheric aerosols and light scattering and extinction in Grand Canyon area[J]. Journal of Geophysical Research,1996, 101:19 251-19 265.

文章导航

/