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数学与物理学

铒单离子磁体(C18H23Er)器件的自旋极化输运

  • 周洁 ,
  • 王正川
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  • 中国科学院大学物理科学学院, 北京 100049

收稿日期: 2017-03-02

  修回日期: 2017-04-11

  网络出版日期: 2018-05-15

基金资助

国家自然科学基金(11274378)和973项目(2013CB933401)资助

Spin-polarized transport through a device of single-ion magnet C18H23Er

  • ZHOU Jie ,
  • WANG Zhengchuan
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  • School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China

Received date: 2017-03-02

  Revised date: 2017-04-11

  Online published: 2018-05-15

摘要

研究单分子磁体的自旋极化输运性质。搭建由扫描隧道显微镜钴针尖、铒单离子磁体以及金(111)衬底所构成的分子器件模型。在小偏压下,计算铒单离子磁体在正立和倒立2种构型下的自旋极化电流曲线,发现此单分子磁体器件的隧穿磁电阻最高达120%,自旋过滤效率在70%~100%。对比2种构型下的整流比,发现倒立构型有较大的整流比。通过分析体系的透射谱、分子投影哈密顿量、器件投影态密度等,对上述物理效应的根源进行解释。

本文引用格式

周洁 , 王正川 . 铒单离子磁体(C18H23Er)器件的自旋极化输运[J]. 中国科学院大学学报, 2018 , 35(3) : 302 -307 . DOI: 10.7523/j.issn.2095-6134.2018.03.003

Abstract

We study the spin-polarized transport through devices of single molecule magnet. A device consisting of the scanning tunneling microscopy Co tip, the single-ion magnet of erbium, and the Au(111) substrate is set up. We calculate the spin-polarized I-V curves for the upward and downward structures of single-ion magnet at a small bias, and find that the tunnel magnetoresistance is as high as 120% and the efficiency of the spin filter at small bias is between 70%-100%. By comparing the spin rectification ratios of the two structures, we find that the downward structure has better spin rectifying effect. Based on the analyses of the transmission spectrum, the molecular projection Hamiltonian, and the projection device density of states, we give reasonable explainations for the above observations.

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